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Just as you would if you had a built-in DVD Optical Disc Drive in your computer, You will need to save the iTunes content on a CD as files in a computer then write then to the LG - 8x External USB Double-Layer DVD±RW/CD-RW Drive - Black, Model # SP80NB80. Not quite clear on what you are looking to do, but the SP80NB80 only connects to a computer via USB. It is compatible with the Windows 10/8.1/8/7/Vista/XP(SP3), and Mac OS X v.10.7.5 or Higher Operating Systems. If you are looking to download iTunes to your iPOD, then you can insert your CD that has the iTunes on it into the SP80NB80 and copy iTunes to your PC/Laptop and if your iPod connects to the PC/Laptop, you can copy them to it. Your PC/Laptop will see the SP80NB80 as another drive & you can copy or move files from it to your PC/Laptop then move those to your iPod if it allows for that. You need to check the manual for your iPod or contact Apple to ask about how to transfer files from a PC/Laptop to the iPod is you're not sure how to do that...^IFV
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