“Anyone know if you can sync documents with a work related Office 365 account?”
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Yes. the ms apps will show both work and personal onedrive folders in the open/save functions. If you have a Work O365 accounts, I'd wonder why you wouldn't just use that account to download the apps on your personal device. I've done that in past.
Sorry, there was a problem. Please try again later.You should be able to sync your files. For more information on syncing files across accounts, follow this link: https://support.office.com/en-us/article/sync-files-with-the-onedrive-sync-client-in-windows-615391c4-2bd3-4aae-a42a-858262e42a49
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