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Hello Joe33! The MK540 Advanced Wireless Keyboard and Mouse Bundle will only work with Windows 10 or later, Windows 8, Windows 7, and Chrome OS, so it won't work with your Toshiba Smart TV no. I'd recommend checking the K600 TV Wireless Keyboard instead, which is a TV Keyboard, and will work with Android TV v6 or later (which I believe Toshiba Smart TV use), here's the link: https://www.bestbuy.com/site/logitech-k600-tv-wireless-keyboard-dark-gray/6282604.p?skuId=6282604
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