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It should. I have Samsung smart TV also and it works fine with it. Should be a complete list of compatibles at Logitech.com.
Sorry, there was a problem. Please try again later.If all your devices are IR compatible then its a good chance the remote will work. What you will do is use the My Harmony app to enter each of your devices then set up a program such as watch TV or watch a movie. I also have two Samsung smart TVs...the remote works just fine.
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